The influence of electric circuit parameters on NOx generation by transient spark discharge
Janda M., Hensel K., Machala Z., Field T. A. J. Phys. D Appl. Phys. 56, 485202, 18 pp, DOI 10.1088/1361-6463/ace634 (2023)
download
|
Abstract: Nitrogen fixation, production of NO and NO2 from N2 and O2 in air, has been investigated with transient spark self-pulsing DC discharges. NO production is boosted by the addition of capacitors and an inductor to the electrical circuit which drives the discharge. The quantity of NO produced per joule of electrical input energy is doubled, though the quantity of NO2 produced drops. The yield of NO is also increased because the modified circuit enables higher discharge currents to be used. NO concentrations as high as 2000 ppm were obtained with input energy densities of around 300 J per litre of input gas, whilst NO2 concentrations were around 150 ppm. This simple modification of the driving circuit may have potential for optimizing the plasma chemistry with other input gas mixtures and for scaling up nitrogen fixation from air.
|
Citations: 1.) | Gulka, M et al. 2024 Surface optimization of nanodiamonds using non-thermal plasma, CARBON 224:119062, 10.1016/j.carbon.2024.119062 (2024) ------------- | 2.) | Abdelaziz, AA et al 2024 Critical Considerations in Power Measurements for the Precise Estimation of Energy Costs in Plasma NOx Synthesis, PLASMA CHEMISTRY AND PLASMA PROCESSING, 10.1007/s11090-024-10472-w (2024) ------------- | 3.) | van Raak, T et al. 2024 Numbering up and sizing up gliding arc reactors to enhance the plasma-based synthesis of NOx, CATALYSIS SCIENCE & TECHNOLOGY, 10.1039/d4cy00655k (2024) ------------- | 4.) | Abdelaziz, A.A., Komuro, A., Teramoto, Y., Schiorlin, M., Kim, D.-Y., Nozaki, T., Kim, H.-H., 2024. Atmospheric-pressure plasmas for NO production: Short review on current status. Current Opinion in Green and Sustainable Chemistry 50, 100977. https://doi.org/10.1016/j.cogsc.2024.100977 (2024) ------------- | 5.) | Zhao, X., 2024. Numerical Study of the Influence of Pressure on the Dynamics and Complex Bifurcation Processes of the Low-Pressure DC Glow Discharge. IEEE Access 12, 116657–116665. https://doi.org/10.1109/ACCESS.2024.3447007 (2024) ------------- | |